I'm assuming your largest ring is a 42T and your largest cog is a 14T?
I'm also assuming your bike has a Freewheel?
That only gives you a gear ratio of 3 to 1, which is about 75 gear inches.
There are 13 tooth FW's available, which would gear you up about 7%, or 81 gear inches.
IF your bike actually has a Free Hub, you have a lot more choices in cassettes, down to 11T top cogs.
http://sheldonbrown.com/free-k7.html