Hey there,
It is nice to see this thread have a spark of life, use to be very active.
Charles Village is decent as is Hampden (Hipster hangout). 2 of my kids live there as do a few friends. One of my kids lives car-free in Hampden. Hampden is nice because it is a true village, stores, restaurants, food stores, hardware etc. Bolton Hill and Mt Vernon are nice places to live as well, close to decent bike infrastructure and great homes. Fells Point and Canton are decent but more ouut of the way and traffic jams.
Post on Bikemore FB site for more info
Balto bike map.
https://transportation.baltimorecity...%29%20rev2.pdf